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Ganglia (bubbles, or droplets) are widespread in porous media of various industrial applications. Thermodynamic properties of a ganglion, including its volume (
In this study, we develop a pore-scale algorithm for determining the morphologies and thermodynamic properties of hydrostatic ganglia in heterogeneous porous media (a 2D pillar array, as illustrated in Figure 1a). Notably, we reveal novel ganglion morphologies: the fluid-fluid interface can emerge between non-adjacent solid particles that do not share a pore unit (referred to as the “cross-pore interface”), although it has long been assumed that a pore is a basic unit of fluid and interface behaviors in porous media [2]. The presence of cross-pore interfaces is strongly associated with the pore-throat ratio: a smaller pore-throat ratio (wider throat) leads to a greater number of metastable morphologies. Interestingly, these novel cross-pore interfaces can also be found in homogeneous media.
We track cycles of quasi-static growth and shrinkage of a ganglion (Figure 1b) and resolve the corresponding thermodynamic properties’ evolution (Figure 1c&d). During growth, the ganglion invades pore by pore, with only one major length scale (the throat) controlling
This work provides insights for investigating quasi-static degassing, ganglia dissolution, and ripening processes, as well as to analyze the thermodynamic stability of dispersed fluid clusters in heterogeneous porous media. In addition, we call for attention that the term “pore” may not always be a valid basic representative unit during the description of fluid and interface behaviors in porous media, as demonstrated by the presence of cross-pore interfaces.
References | 1.Armstrong, R.T., et al., Porous Media Characterization Using Minkowski Functionals: Theories, Applications and Future Directions. Transport in Porous Media, 2018. 130(1): p. 305-335. 2.Wang, C., Y. Mehmani, and K. Xu, Capillary equilibrium of bubbles in porous media. Proceedings of the National Academy of Sciences, 2021. 118(17): p. e2024069118. 3.Li, Y., C. Garing, and S.M. Benson, A continuum-scale representation of Ostwald ripening in heterogeneous porous media. Journal of Fluid Mechanics, 2020. 889. 4.Lin, Q., et al., Drainage Capillary Pressure Distribution and Fluid Displacement in a Heterogeneous Laminated Sandstone. Geophysical Research Letters, 2021. 48(14). 5.Krishnamurthy, P.G., D. DiCarlo, and T. Meckel, Geologic Heterogeneity Controls on Trapping and Migration of CO2. Geophysical Research Letters, 2022. 49(16). |
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Country | China |
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