19–22 May 2025
US/Mountain timezone

A new phase diagram for fluid invasion patterns as a function of pore-scale heterogeneity, surface roughness, and wettability

20 May 2025, 10:05
1h 30m
Poster Presentation (MS06-B) Interfacial phenomena across scales Poster

Speaker

Helmut Geistlinger (UFZ)

Description

Understanding how different flow patterns emerge at various macro- and pore scale heterogeneity, pore wettability and surface roughness is remains a long standing scientific challenge. Such understanding allows to predict the amount of trapped fluid left behind, of crucial importance to applications ranging from microfluidics and fuel cells to subsurface storage of carbon and hydrogen. We examine the interplay of wettability and pore-scale heterogeneity including both pore angularity and roughness, by a combination of micro-CT imaging of 3D grain packs with direct visualization of 2D micromodels. The micromodels are designed to retain the key morphological and topological properties derived from the micro-CT images. Different manufacturing techniques allow us to control pore surface roughness. We study the competition between flow through the pore centers and flow along rough pore walls and corners in media of increasing complexity in the capillary flow regime. The resulting flow patterns and their trapping efficiency are in excellent agreement with previous μ-CT results. We observe different phase transitions between the following flow regimes (phases): (i) Frontal/ compact advance, (ii) wetting and drainage Invasion percolation, and (iii) Ordinary percolation. We present a heterogeneity-wettability-roughness phase diagram that predicts these regimes shown in Fig. 1 (Geistlinger et al., 2024).
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Figure 1. A) The phase diagram shows the transition in flow regimes from A) frontal advance to B) drainage invasion percolation with increasing contact angle and for uniform porous media (2D glass beads). For porous media with higher heterogeneity/disorder and smooth surface (y = 0; Delaunay pore structure, 2D sand) a second transition to wetting invasion percolation is observed. The transitions in displacement regimes are quantified by the finger width, W. B) Phase diagram for porous media with rough surfaces (y > 0).

References Geistlinger, H., Golmohammadi, S., Zulfiqar, B., Kuechler, M., Reuter, D., Schlueter, S., . . . Amro, M. (2024). A new phase diagram for fluid invasion patterns as a function of pore-scale heterogeneity, surface roughness, and wettability. Water Resources Research, 60 (6), e2023WR036036.
Country Germany
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Primary author

Helmut Geistlinger (UFZ)

Co-authors

Bilal Zulfiqar (Helmholtz-Zentrum für Umwelt Forschung- UFZ) Prof. Mohd Amro (Technical University Bergakademie Freiberg, Freiberg, Germany)

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